I'd check out the Merchants of Green just east of the Don Valley Parkway on Queen Street (http://www.merchantsofgreencoffee.com/) as well as Moonbean coffee in Kensington Market. It might also be worth investigating Pilot Coffee Roasters, formerly known as Te Aro, which distributes beans around many indie cafes in Toronto (http://www.pilotcoffeeroasters.com/)
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