In the west end, you can try Butcher by Nature http://www.butcherbynature.com .
There are good butchers in Kensington Market and St. Lawrence Market as well.
If for "GTA" you are willing to travel out of the city, my favourite source for meat is Agram Meats http://www.agrammeats.com/ .
The farm, abattoir, processing, and store are all on the same property near Georgetown, operated by the same people. Not certified organic, (which means their prices are very reasonable) but all natural and local, and I feel good about buying my meat there.
Another not certified organic, but as good as is "Fresh from the Farm" near Donlands and O'Connor. http://freshfromthefarm.ca/. All Kitchener-Waterloo area Mennonite products. Mennonite farmers produce food for their local community, and since they trust each other to use healthy practices, they don't feel the need to certify. Good stuff, available in store or by pre-order. Also baked goods, home canning, cheese, eggs and produce (in season).
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